Condensed matter theory

Moiré materials host fractional Chern insulators and electron crystals in close proximity, but the mechanism selecting between them remains an open question. We address this competition in Chern bands with ideal but momentum-dependent quantum geometry -- Aharonov-Casher bands. We present an ansatz wave function for generalized Wigner crystals and, by comparing its energy to that of the competing Laughlin-like state, map out the phase diagram at filling fraction $ν=1/m$ as a function of the degree of geometric non-uniformity. Our work identifies quantum geometry-controlled zero point fluctuations of the charge density of the generalized Wigner crystal as the mechanism controlling its relative stability, implying a kind of quantum Lindemann criterion for the crystal-liquid phase boundary.

Colloidal quantum dot (cQD) thin films are central to solution-processed optoelectronics, yet scalable deposition methods that preserve device performance while improving material utilization remain limited. Here, we adapt a biphasic meniscus dip coating strategy that enables controlled deposition of cQD films while substantially reducing the volume of active nanocrystal solution required. In this approach, a thin cQD layer is supported by an immiscible underlayer, such that film formation occurs exclusively at the liquid-air interface of the active phase. Using this geometry, we fabricate PbS quantum dot photodetectors with responsivities up to ∼1000 mA/W at 1200 nm, comparable to conventional spin-coated devices. Relative to spin coating, the biphasic configuration reduces active solution consumption by up to 20-fold while maintaining film quality and reproducible device performance. A mass-volume cost analysis shows that the reduced active reservoir shifts the economic viability of dip coating into thickness and throughput regimes more relevant to practical device fabrication. We further extend the method to CsPbBr3 nanocrystals and curved substrates, highlighting its generality across material systems and geometries. Together, these results establish biphasic dip coating as a material-efficient and device-compatible manufacturing strategy for solution-processed optoelectronics.

Abstract The idea that topologically protected quantum states, such as anyons, may be attached to super/semiconductor heterostructures has received enormous attention, but experimental signatures in 1D systems remain elusive. Here we revisit theoretical underpinnings of anyons in 2D fractional quantum Hall (FQH) systems, whose signatures have been experimentally observed by independent groups. We highlight novel theorems about the Hopfion or CP 1-model, understood as quantization of FQH surplus flux in 2-Cohomotopy, which retrodicts abelian FQH anyon properties in fine detail. Examining this theoretical model further, we find that islands of expelled flux enlarge the ground-state monodromy from an abelian group to a (framed spherical) braid group, nonabelian for two or more islands, so that nonabelian anyonic states become topologically admissible; superconducting islands are one candidate realization of such flux expulsion.

Spin-orbit torque (SOT) provides an efficient route for manipulating magnetization in spintronic devices, and its accurate quantification is essential. Here, we investigate Co/Gd-based synthetic ferrimagnets using complementary magnetotransport and magneto-optical techniques. We use a Sagnac magneto-optical interferometry method to directly quantify current-induced magnetization tilting and extract the damping-like SOT effective field. The Sagnac measurements show good agreement with harmonic Hall analysis across different Co/Gd and Gd/Pt/Co heterostructures, providing a quantitative determination of the damping-like SOT effective field that does not rely on electrical transport signatures. By varying the Gd thickness and multilayer stacking order, we demonstrate that the damping-like torque is strongly influenced by spin transport and angular momentum conversion at rare-earth and heavy-metal interfaces. The observation of a finite torque in Gd/Pt/Co/Pt structures, where conventional Pt spin Hall contributions are expected to compensate, highlights the active role of the Gd layer in SOT generation. Furthermore, interface engineering enables perpendicular magnetic anisotropy in Gd/Pt/Co/Al heterostructures with a 2-nm-thick Co layer, allowing current-induced SOT switching at current densities of 8-10 MA/cm². These results establish rare-earth-based synthetic ferrimagnets as a versatile platform for engineering spin-orbit phenomena and optimizing low-power spintronic devices.

In this work, we demonstrate the oriented growth of quasi-2D metal halide perovskite nanowire and nanoplate arrays with continuous corner-sharing metal halide octahedra sheets normal to the substrate surface, the optimal orientation for device stacks. Oriented perovskite growth is achieved through two-step deposition in TiO 2 nanoporous scaffolds in which PbI 2 films are immersed in co-solutions of formamidinium iodide (FAI) and n-butylammonium iodide (BAI) in isopropyl alcohol to form metal halide perovskites. At 50 mol% FAI or higher relative to BAI, only 3D FAPbI 3 (n = ∞) nanowires form at room temperature. BAI does not incorporate into the crystal lattice at these concentrations but stabilizes semiconducting α-FAPbI 3 from converting to insulating δ-FAPbI 3, the thermodynamically stable phase at room temperature. Immersion in solutions with 33 mol% FAI or lower results in quasi-2D (BA) 2 (FA)Pb 2 I 7 (n = 2) or 2D (BA) 2 PbI 4 (n = 1) nanoplate growth. In situ photoluminescence spectra collected during crystal growth revealed the presence of intermediate n >2 phases before conversion to the thermodynamically favored phase at some compositions. Vertical gradients in n number were also identified by monitoring photoluminescence from the tops and bottoms of films, with α-FAPbI 3 and low n phases preferentially forming at the film surfaces and buried interfaces, respectively. Proof-of-concept conductivity mapping via atomic force microscopy demonstrates that these compositionally-graded nanocrystalline arrays are photoconductive, with highest conductivity normal to the substrate.

Topological Anderson insulators provide a paradigm for disorder-induced topology, in which the underlying system turns from a trivial to a topological phase. It is widely recognized that the latter disappears at large disorder amplitude. Here, and contrary to the general belief, we provide evidence for successive disorder-driven topological transitions ending up in an unconventional topological Anderson phase that remains unexpectedly robust at strong disorder. The corresponding topological invariant increases stepwise with disorder, and then saturates in the strong-disorder regime, without reverting to a trivial Anderson insulator. We experimentally realize these topological Anderson staircase transitions in a one-dimensional topolectrical circuit that emulates single-wall nanotubes. Our work opens the road to topological disordertronics, in which robust topological phases can be tuned by disorder. Using a topolectrical circuit, the authors realise an unconventional disorder-tuned cascade of topological Anderson phase transitions ending up, contrary to the general belief, in an extremely robust topological phase. This work opens the gate for topological disordertronics, where topological channels can be tuned by disorder.

The superconducting diode effect is an asymmetry in the critical current with respect to the supercurrent polarity. One impetus driving recent interest in the effect is its dependence on intrinsic or microscopic symmetry breaking mechanisms. Here, we study the superconducting diode effect in gated planar Josephson junctions fabricated on a superconductor--semiconductor heterostructure under an in-plane magnetic field. We observe two gate-driven inversions of the diode polarity in the vicinity of zero field, as well as a third-harmonic component in the dependence of the diode efficiency on the in-plane field angle. We analyze the Lifshitz invariant for an arbitrary spin--orbit coupling and show that multiple polarity inversions are possible in the presence of both linear and cubic Dresselhaus terms, where the Rashba parameter varies monotonically with gate voltage. Numerical calculations of the diode efficiency further reveal the presence of higher harmonics in its field-angle dependence in the presence of spin--orbit coupling.

Random circuits giving rise to unitary designs are key tools in quantum information science and many-body physics. In this work, we investigate a class of random quantum circuits with a specific gate structure. Within this framework, we prove that one-dimensional structured random circuits with non-Haar-random local gates can exhibit substantially more global randomness compared to Haar-random circuits with the same underlying circuit architecture. In particular, under a solvability condition, we exactly diagonalize the second-moment operators for these structured random circuits by establishing a link to free-fermionic models, and we show that their spectral gaps can exceed those of Haar-random circuits. While solvable structured random circuits exhibit free-fermionic behavior, the underlying fixed gate need not be a matchgate. Our findings have applications in improving circuit depth bounds for randomized benchmarking, in generating approximate unitary 2-designs from shallow random circuits, and in enabling exact analyses of quantum many-body dynamics.

High Resolution Image Download MS PowerPoint Slide Poly(phenylenevinylene)s (PPV)s are a class of fluorescent conjugated polymers used in organic light emitting diodes (OLEDs). Living chain growth polymerization of PPVs is typically achieved by ring-opening metathesis polymerization (ROMP) of highly strained cyclophanedienes. While benzene-based cyclophanedienes are routinely reported, living or controlled ROMP of naphthalene-benzene containing mixed cyclophanedienes remains a challenge. This work describes the synthesis and polymerization of an alkoxy substituted naphthalene-benzene cyclophanediene using Schrock’s molybdenum olefin metathesis catalyst. We demonstrate the efficacy of this strategy in producing poly(naphthalene benzene vinylene) (PNBV)s with controlled molecular weights and narrow dispersities. The produced PNBVs are highly fluorescent polymers in solution and as thin films with distinct emission signatures arising from the benzene and naphthalene chromophores. An unoptimized PNBV thin film transistor exhibited a hole mobility of 8 × 10 –9 cm 2 /V·s, which increased to 1 × 10 –7 cm 2 /V·s upon doping with lithium bis(trifluoromethanesulfonyl) imide (LiTFSI) and (tris(2-(1 H-pyrazol-1-yl)-4- tert-butylpyridine)cobalt(III) (FK 209). This expansion of ROMP to include the naphthalene moiety as well as a mixed-aromatic system will usher further development of electronically diverse PPVs with advanced solid-state applications.

Semiconductor crosshatch patterns form as a result of strain relaxation and dislocation pileups during growth of lattice mismatched materials. Due to their connection with the internal misfit dislocation network, these patterns are a complex fingerprint of internal strain relaxation and growth anisotropy. Therefore, these patterns not only describe the residual strain state at the surface, but could also provide an indicator of electron transport quality through the material. Here, we present a method utilizing computer thresholding and machine learning to analyze antiferromagnetic (AFM) crosshatch patterns that exhibits this correlation. Our analysis reveals optimized electron transport for moderate values of λ (crosshatch wavelength) and ε (crosshatch height), roughly 1 m and 4 nm, respectively, that define the average wave form of the pattern. Simulated two-dimensional AFM crosshatch patterns are used to train a machine learning model to correlate the crosshatch patterns to dislocation density. This model is used to evaluate the experimental AFM images and predict a dislocation density based on the crosshatch wave form. Predicted dislocation density, experimental AFM crosshatch data, and transport measurements are used to train a final model to predict electron mean free path. Our model shows electron scattering is dominated by elastic effects (e.g., dislocations) below 150 nm λMFP.

Nearly a century after Wigner's initial proposal, electron crystals are now a topic of intense experimental and theoretical interest. However, most proposed crystalline phases are commensurate and therefore become insulating in the presence of even weak pinning. In this work we discuss when a commensurate Wigner crystal will spontaneously self dope and develop itinerant carriers, giving rise to an incommensurate and thus metallic Wigner crystal (MWC). We develop a general criterion for the instability of the commensurate crystal which involves the competition between the charge gap at commensurability and a ``packing bias'' whose sign selects whether electron or hole doping is preferred. We then apply these insights to rhombohedral multilayer graphene, where calculations for commensurate crystals reveal instabilities towards self-doping. Carrying out self-consistent Hartree-Fock over the landscape of incommensurate crystals reveals the phase diagram, where a broad MWC phase appears directly adjacent to an insulating Wigner crystal phase. Recent observations of an island of reversed Hall conductance near a putative Wigner crystal phase in rhombohedral graphene are naturally explained by our theory.

Abstract Collective excitations of Fractional Quantum Hall (FQH) liquids at long wavelengths are thought to be of a generally covariant geometric nature, governed by area-preserving diffeomorphisms (SDiff). But current analyses rely solely on the corresponding perturbative w ∞ Lie algebra. We argue this is insufficient: We identify a non-perturbative construction of the effective Maxwell-Chern-Simons quantum field theory which carries unitary SDiff equivariance. But this turns out to be non-differentiable, suggesting underappreciated subtleties when the usual Hilbert space truncation is removed.

We investigate a coherently driven exciton–photon microcavity with Kerr nonlinearity in the ultrastrong-coupling regime. When the lower and upper polariton branches are well separated in energy, the full Hopfield–Rabi–Kerr model reduces to an effective single-mode description of the lower polariton. We analyze the stability of the lower-polariton steady states. We show that the resulting bistability is qualitatively similar to that in the strong-coupling regime. However, in the ultrastrong-coupling regime counter-rotating processes and the diamagnetic A 2 term renormalize the polariton spectrum and composition, changing the effective detuning Δ ̃ 1 and nonlinearity U LP g-dependency beyond the strong-coupling (RWA) picture. As a result, although the semiclassical bistability criterion keeps its standard Kerr-oscillator form, the turning points and hysteresis window are shifted relative to the strong-coupling prediction.

The idea that topologically protected quantum states, such as anyons, may be attached to super/semiconductor heterostructures has received enormous attention, but experimental signatures in 1D systems remain elusive. Here we revisit theoretical underpinnings of anyons in 2D fractional quantum Hall (FQH) systems, whose signatures have been experimentally observed by independent groups. Invoking novel theorems about the Hopfion or CP¹-model understood as flux quantization in 2-Cohomotopy, we demonstrate a robust prediction for possibly nonabelian anyonic states induced by superconducting islands.

Recent advances in moiré engineering motivate the study of lattice models of strongly-correlated electrons subjected to substantial orbital magnetic flux. We analyze the triangular lattice Hofstadter-Hubbard model at one-quarter flux quantum per plaquette and a density of one electron per site, where a chiral spin liquid phase may exist between weak-coupling integer quantum Hall and strong-coupling 120∘ antiferromagnetic phases. We use matrix product state methods and analytical arguments to investigate this model compactified to cylinders of finite circumference. We uncover a glide particle-hole symmetry operation which, we argue, is spontaneously broken at the quantum Hall to spin liquid transition on odd-circumference cylinders. We numerically verify the spontaneous symmetry breaking and further demonstrate that this transition is associated with algebraic long-range correlations of various spin-singlet, charge-neutral operators. For even-circumference cylinders, the transition becomes a crossover associated with a large correlation length that grows substantially with circumference. Our findings suggest that in the two-dimensional limit, the transition to a chiral spin liquid phase is continuous and features critical fluctuations of the current.

Collective excitations of Fractional Quantum Hall (FQH) liquids at long wavelengths are thought to be of a generally covariant geometric nature, governed by area-preserving diffeomorphisms (SDiff). But current analyses rely solely on the corresponding perturbative w∞ Lie algebra. We argue this is insufficient: We identify a non-perturbative construction of the effective Maxwell-Chern-Simons quantum field theory which carries unitary SDiff equivariance. But this turns out to be non-differentiable, suggesting underappreciated subtleties when the usual Hilbert space truncation is removed.

One-dimensional topological Anderson insulators provide a paradigm for disorder-induced topological phases in which the underlying system turns from a trivial to a topological phase. It is widely recognized that the latter vanishes at large disorder amplitude. Here, and contrary to the general belief, we provide evidence for a successive disorder-driven topological transitions in a single-wall nanotube, culminating in a topological Anderson phase that remains unexpectedly robust at strong disorder. This phenomenon is confirmed by analysis of the corresponding topological invariant, which increases stepwise as disorder increases, giving evidence for the emergence of edge states. We experimentally implement these topological Anderson staircase phase transitions in a one-dimensional topolectrical circuit, where the persistence of edge states is revealed by node-voltage measurements. The robustness of the edge states is corroborated by numerical calculations of their localization properties. Our work opens the road to topological disordertronics, where topological phases can be tuned by disorder.

ABSTRACT Optically active tetrathiafulvalene (TTF) banded spherulite films comprising helicoidal fibrils exhibit an order of magnitude higher hole mobility compared to their unbanded counterparts. These mobilities of ∼10 −5 cm 2 V −1 s −1 are, however, low among organic semiconductors. We enhance the electrical conductivity of TTF banded spherulite films over seven orders of magnitude by iodine doping. Pale yellow films became dark red as TTF + formed in the presence of iodine vapor, with the local doping rate dependent on the crystal face exposed at the film surface. A six‐order‐of‐magnitude increase in conductivity is observed during the first two min of doping, reaching a maximum value of 0.7 ± 0.6 S cm −1 after 10 min. TTF 7 I 5 needles nucleated at the film surface and grew downwards during iodine vapor exposure, consuming β‐TTF helicoidal fibrils. The four principal linear optical anisotropies, linear and circular birefringence and dichroism, are mapped, and all four properties decreased over 10 min of iodine vapor exposure due to conversion to TTF 7 I 5. For short doping times, however, circular birefringence and dichroism remained unchanged. These results demonstrate that the conductivity of TTF banded spherulite films can be increased without disrupting the microstructure that gives rise to optical activity, expanding their utility in chiroptoelectronics.

The gatemon qubits, made of transparent superconducting-semiconducting Josephson junctions, typically have even weaker anharmonicity than the opaque AlOx-junction transmons. However, flux-frustrated gatemons can acquire a much stronger anharmonicity, originating from the interference of the higher-order harmonics of the supercurrent. Here we investigate this effect of enhanced anharmonicity in split-junction gatemon devices based on InAs-Al 2D heterostructure. We find that anharmonicity in excess of 100% can be routinely achieved at the half-integer flux sweet-spot without any need for electrical gating or excessive sensitivity to the offset charge noise. We verified that such intrinsically large anharmonicity enables our devices to be driven coherently with raw Rabi frequencies exceeding 100 MHz, without any pulse shaping, simplifying implementation and control compared to traditional gatemons and transmons. Furthermore, by analyzing a relatively high-resolution spectroscopy of the device transitions as a function of flux, we were able to extract fine details of the current-phase relation, to which transport measurements would hardly be sensitive. The strong anharmonicity of our anharmonic tunable transmons, along with their bare-bones design, can prove to be a precious resource that transparent superconducting-semiconducting junctions bring to quantum information processing.

The promise of tantalum for realizing superconducting quantum devices has generated interest in its compound films, particularly nitrides. Among these, cubic-phase tantalum carbonitride (TaCxN1−x) offers reduced susceptibility to oxidation and a high critical temperature, yet its microwave properties remain largely unexplored. Here, we investigate plasma-enhanced atomic layer deposition of cubic-phase TaCxN1−x thin films for superconducting microwave circuits. Structural and transport measurements reveal nanocrystalline morphology with sub-10 nm grains and superconductivity in the dirty limit. Coplanar waveguide resonators exhibit moderately high kinetic inductance (16.8 pH/sq for 30 nm films) with potential for enhancement through dimensional scaling. The films also support high internal quality factors exceeding 105 at 50 mK in the single-photon regime, comparable to granular aluminum. Loss analysis identifies the two-level systems as the dominant limiting mechanism, with potential for further reduction through interface engineering. These results establish atomic layer deposited TaCxN1−x as a promising material for scalable, low-loss, high-inductance superconducting circuits.

Doping-induced superconductivity in group-IV elements may enable quantum functionalities in material systems accessible with well-established semiconductor technologies. Non-equilibrium hyperdoping of group-III atoms into C, Si or Ge can yield superconductivity; however, its origin is obscured by structural disorder and dopant clustering. Here we report the epitaxial growth of hyperdoped Ga:Ge films and trilayer heterostructures by molecular-beam epitaxy with extreme hole concentrations (nh = 4.15 × 1021 cm−3, 17.9% Ga substitution) that yield superconductivity with a critical temperature of Tc = 3.5 K. Synchrotron-based X-ray absorption and scattering methods reveal that Ga dopants are substitutionally incorporated within the Ge lattice, introducing a tetragonal distortion to the crystal unit cell. Our findings, corroborated by first-principles calculations, suggest that the structural order of Ga dopants creates a narrow band for the emergence of superconductivity in Ge, establishing hyperdoped Ga:Ge as a low-disorder, epitaxial superconductor–semiconductor platform. The epitaxial growth of hyperdoped Ga:Ge films and trilayer heterostructures by molecular-beam epitaxy yield superconductivity with a critical temperature of 3.5 K and may enable quantum functionalities in this material system, which is accessible with well-established semiconductor technologies.

We study symmetry preserving adiabatic and Floquet dynamics of one-dimensional systems. Using quasiadiabatic evolution, we establish a correspondence between adiabatic cycles and invertible defects generated by spatially truncated Thouless pump operators. Employing the classification of gapped phases by module categories, we show that the Thouless pumps are classified by the group of autoequivalences of the module category. We then explicitly construct Thouless pump operators for minimal lattice models with VecG, Rep($G$), and Rep($H$) symmetries, and show how the Thouless pump operators have the group structure of autoequivalences. The Thouless pump operators, together with Hamiltonians with gapped ground states, are then used to construct Floquet drives. An analytic solution for the Floquet phase diagram characterized by winding numbers is constructed when the Floquet drives obey an Onsager algebra. Our approach points the way to a general connection between distinct Thouless pumps and distinct families of Floquet phases.

The jellium model is a paradigmatic problem in condensed matter physics, exhibiting a phase transition between metallic and Wigner crystal phases. However, its vanishing Berry curvature makes it ill suited for studying recent experimental platforms that combine strong interactions with nontrivial quantum geometry. These experiments inspired the anomalous Hall crystal (AHC)-a topological variant of the Wigner crystal. The AHC spontaneously breaks continuous translation symmetry but has a nonzero Chern number. In this Letter, we introduce λ-jellium, a minimal extension of the two-dimensional jellium model. Its Berry curvature distribution is controlled by a single parameter λ, where λ=0 corresponds to the standard jellium model. This setup facilitates the systematic exploration of Berry curvature's impact on electron crystallization. The phase diagram of this model, established using self-consistent Hartree Fock calculations, reveals several interesting features: (i) The AHC phase occupies a large region of the phase diagram. (ii) Two distinct Wigner crystal phases, the latter enabled by quantum geometry, and two distinct Fermi liquid phases are present. (iii) A continuous phase transition separates the AHC and one of the Wigner crystal phases. (iv) In some parts of the AHC phase, the lattice geometry is nontriangular, unlike in the classical Wigner crystal. In addition to elucidating the physics of correlated electrons with nonzero Berry curvature, we expect that the simplicity of the model makes it an excellent starting point for more advanced numerical methods.

Thin films of vanadium silicide (V-silicide) in the A15 cubic phase (V3Si) are promising for superconducting quantum devices due to their high transition temperature and potential compatibility with scalable semiconductor fabrication. However, solid-phase synthesis often yields secondary silicide phases that degrade performance. Here, we investigate the influence of substrate properties using two silicon-on-insulator architectures: one with a polycrystalline HfO2 buried layer (group A) and the other with amorphous SiO2 (group B). Both systems exhibit superconductivity consistent with V3Si formation, yet structural analysis reveals mixed-phase films in both cases. Crucially, only group A maintains an atomically sharp and chemically stable interface, a prerequisite for phase purity. Prolonged annealing in group A reduces the unwanted V5Si3 phase but also leads to the emergence of Si-rich VSi2, likely due to localized substrate degradation. Preliminary atomic-resolution imaging suggests that HfO2 crystallinity may promote local phase-selective nucleation. These findings highlight the importance of substrate design in promoting phase control and maintaining interfacial integrity in superconducting silicides.

Recent advances in 2D materials featuring nonzero Berry curvature have inspired extensions of the Wigner crystallization paradigm. This paper derives a low-energy effective theory for such quantum crystals, including the anomalous Hall crystal (AHC) with nonzero Chern number. First, we show that the low frequency dispersion of phonons in AHC, despite the presence of Berry curvature, resembles that of the zero field (rather than finite magnetic field) Wigner crystal due to the commutation of translation generators. We explain how key parameters of the phonon theory such as elastic constants and effective mass can be extracted from microscopic models, and apply them to two families of models: the recently introduced [Formula: see text]-jellium model and a model of rhombohedral multilayer graphene (RMG). In the [Formula: see text]-jellium model, we explore the energy landscape as crystal geometry shifts, revealing that AHC can become "soft" under certain conditions. This causes transitions in lattice geometry, although the quantized Hall response remains unchanged. Surprisingly, the Berry curvature seems to enhance the effective mass, leading to a reduction in phonon speed. For the AHC in RMG, we obtain estimates of phonon speed and shear stiffness. We also identify a previously overlooked "kineo-elastic" term in the phonon effective action that is present in the symmetry setting of RMG, and leads to dramatic differences in phonon speeds in opposite directions. We numerically confirm these predictions of the effective actions by time-dependent Hartree-Fock calculations.

Demonstrating superconductivity in purely repulsive Hubbard models is a compelling goal which underscores the counter-intuitive ability of Coulomb interactions to mediate superconductivity. Here, we present numerical evidence for robust superconductivity in a triangular Hubbard-Hofstadter model at $π/2$ flux per plaquette. Employing infinite density matrix renormalization group calculations on infinite cylinders of finite circumference, we observe superconducting ground states for a wide range of dopings, whose pair-correlations strengthen as the 2D limit is approached. At a density of one electron per site, Hubbard interactions have been reported to drive the insulating parent state of the superconductor from an integer quantum Hall (IQH) state to a chiral spin liquid (CSL). Our findings give credence to a recent proposal that proximity to the IQH-CSL transition serves to make chiral superconductivity energetically favorable on doping, and also correctly predicts the nature of the edge modes in the superconductor. On the CSL side, this suggests the superconductor can be thought of as arising from Laughlin's `anyon superconductivity' mechanism. Thus the Hubbard-Hofstadter model studied here offers a clean and experimentally accessible setup, potentially realizable in moiré heterostructures, for exploring the properties of anyonic matter at finite density and the interplay of topological order, quantum criticality and superconductivity.

We argue that the combination of strong repulsive interactions and high magnetic fields can generate electron pairing and superconductivity. Inspired by the large lattice constants of moiré materials, which make large flux per unit cell accessible at laboratory fields, we study the triangular lattice Hofstadter-Hubbard model at one-quarter flux quantum per plaquette, where previous literature has argued that a chiral spin liquid separates a weak-coupling integer quantum Hall phase and a strong-coupling topologically trivial antiferromagnetic insulator at a density of one electron per site. We argue that topological superconductivity emerges upon doping in the vicinity of the integer quantum Hall to chiral spin liquid transition. We employ exact diagonalization and density matrix renormalization group methods to examine this theoretical scenario and find that electronic pairing indeed occurs on both sides of criticality over a remarkably broad range of interaction strengths. On the chiral spin liquid side, our results provide a concrete model realization of the long-hypothesized mechanism of anyon superconductivity. Our study thus establishes a beyond-Bardeen-Cooper-Schrieffer route to electron pairing in a well-controlled limit, relying crucially on the interplay between electron correlations and band topology.

Operator spreading under stroboscopic time evolution due to a unitary is studied. An operator Krylov space is constructed and related to orthogonal polynomials on a unit circle (OPUC), as well as to the Krylov space of the edge operator of the Floquet transverse field Ising model with inhomogeneous couplings (ITFIM). The Verblunsky coefficients in the OPUC representation are related to the Krylov angles parameterizing the ITFIM. The relations between the OPUC and spectral functions are summarized and several applications are presented. These include derivation of analytic expressions for the OPUC for persistent $m$-periodic dynamics, and the numerical construction of the OPUC for autocorrelations of the homogeneous Floquet-Ising model as well as the Z3 clock model. The numerically obtained Krylov angles of the Z3 clock model with long-lived period tripled autocorrelations show a spatial periodicity of six, and this observation is used to develop an analytically solvable model for the ITFIM that mimics this behavior.

The discovery of fractional quantum anomalous Hall states in moiré systems has raised the possibility of realizing phases of itinerant anyons, whose mobility requires the absence of continuous magnetic translation symmetry (CMTS). Motivated by this, we consider anyons on the sphere in the presence of a nonuniform magnetic field that breaks the SU(2) rotation symmetry, the analog of CMTS on the sphere, down to a U(1). This allows us to study the energy dispersion of the anyons as a function of the angular momentum L_{z}, while maintaining the perfect flatness of the single-particle dispersion. We parametrize the nonuniform field by a real parameter R that concentrates the field at the north (south) pole for R>1 (R<1). For this choice of field, any p-body correlation function evaluated in the space of Laughlin quasiholes maps exactly onto the corresponding p-body correlation function in uniform field. In the thermodynamic limit, this exact mapping lets us analytically compute the interaction-generated, spatially varying potential felt by the anyons. Remarkably, this static potential alone is sufficient to generate anyon dispersion: because each anyon experiences an emergent background magnetic field, the two components of its position do not commute, so the potential is converted into a finite dispersion, which we compute exactly up to an overall scaling constant. The resulting anyon dispersion describes the azimuthal motion around the sphere at constant height, the analog of spin precession. Our Letter thus provides an exactly solvable realization of a general mechanism for interaction-induced anyon dispersion-a symmetry-breaking potential converted into kinetic energy by the anyon's many-body Berry phase-with no single-particle dispersion or hopping of any kind.

Interacting fermionic chains exhibit extended regions of topological degeneracy of their ground states as a result of the presence of Majorana or parafermionic zero modes localized at the edges. In the opposite limit of infinite temperature, the corresponding nonintegrable spin chains, obtained via generalized Jordan-Wigner mapping, are known to host so-called almost strong zero modes, which are long-lived with respect to any bulk excitations. Here we study the fairly unexplored territory that bridges these two extreme cases of zero and infinite temperature. We blend two established techniques for states, the Lanczos series expansion and a tensor network ansatz, uplifting them to the level of operator algebra. This allows us to efficiently simulate large system sizes for arbitrarily long timescales and to extract the temperature-dependent decay rates. We observe that for the Kitaev-Hubbard model, the decay rate of the edge mode depends exponentially on the inverse temperature β, and on an effective energy scale Δ eff that is greater than the thermodynamic gap of the system Δ.

Topology has emerged as a field for describing and controlling order and matter, and thereby the physical properties of materials. There are several largely disparate fields focused on examining and manipulating topology. One of these arenas is in the realm of real space, manipulating systems in terms of their spatial properties, to control the corresponding structural, mechanical, and self- assembling responses. Much of the work in soft matter topology falls within this domain. A second arena is in the domain of momentum or k-space wherein topology controls the features of the electronic band structure of materials, and topologically non-trivial features result in the development of materials with truly unique properties. This work focuses squarely on the realm of condensed matter physics. Here, we review concepts of real- and k-space topology and propose areas for convergence between these two disparate fields.

The authors investigate here light-induced Dirac-to-Weyl conversion in the massive 3D Dirac semimetal Co3Sn2S2 via ultrafast mid-infrared pump--terahertz probe Faraday rotation spectroscopy. The observed anomalous Hall conductivity under circularly polarized light shows electric field and driving frequency dependence consistent with Floquet-induced Berry curvature from Dirac band splitting. The estimated splitting reaches ~60% of the mass gap, and a theoretical calculation based on Floquet theory quantitatively reproduces the experimental observation, highlighting a promising approach for realizing Floquet-Weyl states in gapped 3D Dirac systems.

Abstract We study the kinetic Ising model under Glauber dynamics and establish an upper bound on the spectral gap for finite systems. This bound implies the critical exponent inequality z ≥ 2 z ≥ 2, thereby rigorously improving the previously known estimate z ≥ 2 - η z ≥ 2 - η. Our proof relies on the mapping from stochastic processes to frustration-free quantum systems and leverages the Simon–Lieb and Gosset–Huang inequalities.

Abstract The rational design of molecular electronics remains a grand challenge of materials science. DNA nanotechnology has offered unmatched control over molecular geometry, but direct electronic functionalization is a challenge. Here a generalized method is presented for tuning the local band structure of DNA using transmetalation in metal‐mediated base pairs (mmDNA). A method is developed for time‐resolved X‐ray diffraction using self‐assembling DNA crystals to establish the exchange of Ag + and Hg 2+ in T:T base pairs driven by pH exchange. Transmetalation is tracked over six reaction phases as crystal pH is changed from pH 8.0 to 11.0, and vice versa. A detailed computational analysis of the electronic configuration and transmission in the ensuing crystal structures is then performed. This findings reveal a high conductance contrast in the lowest unoccupied molecular orbitals (LUMO) as a result of metalation. The ability to exchange single transition metal ions as a result of environmental stimuli heralds a means of modulating the conductance of DNA‐based molecular electronics. In this way, both theoretical and experimental basis are established by which mmDNA can be leveraged to build rewritable memory devices and nanoelectronics.

In the accompanying paper [Y. Mitsuhashi, et al., Phys. Rev. Lett. 134, 180404 (2025)], we established the method of characterizing the maximal order of asymptotic unitary designs generated by symmetric local random circuits, and explicitly specified the order in the cases of Z2, U(1), and SU(2) symmetries. Here, we provide full details on the derivation of the main theorems for general symmetry and for concrete symmetries. Furthermore, we consider a general framework where we have access to a finite set of connected compact unitary subgroups, which includes symmetric local unitary gate sets.

We have established the method of characterizing the unitary design generated by a symmetric local random circuit. Concretely, we have shown that the necessary and sufficient condition for the circuit asymptotically forming a t-design is given by simple integer optimization for general symmetry and locality. By using the result, we explicitly give the maximal order of unitary design under the Z_{2}, U(1), and SU(2) symmetries for general locality. This work reveals the relation between the fundamental notions of symmetry and locality in terms of randomness.

High Resolution Image Download MS PowerPoint Slide Ferrimagnetic insulators with ultralow damping are of great interest for their potential applications in energy-efficient computing devices. Here, we report the direct electrical detection of magnetic auto-oscillations in unpatterned ultralow damping ferrimagnetic insulator epitaxial Li 0.5 Al 0.5 Fe 2 O 4 thin films, driven by a current in a proximal Pt nanowire. Auto-oscillations occur for only one current polarity, consistent with the spin-Hall effect inducing the oscillation state. Micromagnetic modeling shows good agreement with the experimental frequency and field dispersions, showing only one dominant oscillation mode, in contrast to the multiple modes typically observed in transition-metal nanowire-type spin-Hall nanooscillators. This study illustrates a new material system for neuromorphic computing and magnonics, a simple material platform with the direct-current generation of high-frequency (∼10 GHz) signals and their electrical detection.

We demonstrate the possibility of covalently bonded hybrid DNA–graphene materials by synthesizing a model DNA–polycyclic aromatic hydrocarbon (PAH) conjugate comprising a 33mer oligonucleotide containing thymine and uridine modified with bispyrenyl benzene. This DNA–PAH conjugate (T 13 U PAH T 19; T = thymine, U PAH = PAH-modified uridine) has an atomically thin nanographene protrusion extending by only about 1 nm from the single-stranded DNA (ssDNA). We show that DNA–PAH conjugates can be characterized with high resolution by profiling with a nanopore in a monolayer MoS 2 membrane. The profiling experiments provided sufficient resolution to distinguish the thymine and PAH-modified regions of T 13 U PAH T 19 and confirm the asymmetry of the PAH attachment relative to the 3′ and 5′ ends of the ssDNA due to different lengths of the T 13 and T 19 segments. This work provides the foundation for further exploration of DNA–graphene hybrids, demonstrating an example of their synthesis and the utility of nanopore profiling for their structural characterization with an ∼1 nm resolution.

By coupling a semiconductor-based planar Josephson junction to a superconducting microwave resonator, we investigate the Andreev bound states in the junction using dispersive readout techniques. Using electrostatic gating to create a narrow constriction in the junction, our measurements unveil a strong coupling interaction between the resonator and the Andreev bound states. This enables the mapping of isolated tunable Andreev bound states that can reach near-unity transparency along with an average induced superconducting gap of ∼ 150 µ eV. Exploring the gate parameter space further elucidates a nonmonotonic evolution of multiple Andreev bound states with varying gate voltage. Complementary tight-binding calculations of an Al-InAs planar Josephson junction with strong Rashba spin-orbit coupling provide insight into possible mechanisms responsible for such behavior. Our findings highlight the subtleties of the Andreev spectrum of Josephson junctions fabricated on superconductor-semiconductor heterostructures, offering potential applications in probing topological states in these hybrid platforms.

High Resolution Image Download MS PowerPoint Slide Engineering the electronic band structure of two-dimensional (2D) materials by imposing spatially periodic superlattice (SL) potentials opens a pathway to unconventional electronics. Nanopatterning the gate electrode or surface dielectric near 2D crystals provides a powerful strategy for realizing electrostatically tunable “remote” SLs with flexibility in lattice design. Here, we demonstrate the effectiveness of block copolymer (BCP)-templated dielectric nanopatterns for fabricating etch-free high-grade metal oxide SLs. Alumina (AlO x) nanopatterns with hexagonal symmetry and a 38 nm SL wavelength are produced as a model material by directly converting a self-assembled BCP film via block-selective vapor phase infiltration. Despite micrometer-scale rotational disorder inherent to BCP self-assembly, electronic transport measurements of graphene reveal replica Dirac points at zero field and Hofstadter mini-gaps under finite magnetic fields. These results indicate the successful formation of remote SL potentials in graphene resulting from optimized AlO x nanopattern fabrication to achieve consistent lattice symmetry and periodicity at a macroscopic scale. The findings of this study, combined with the versatile, scalable, and cost-effective nature of BCP nanopatterning, highlight the potential of BCP-templated nanostructures for remote SL engineering in 2D crystals.

Single molecules bridging two metallic electrodes can emit light through electroluminescence when subjected to a bias voltage. Typically, light emission in such devices results from transitions between molecular states, although in the presence of light-matter coupling, the emission can result from a transition between hybrid light-matter states. Here, we create single metal-molecule-metal junctions and simultaneously collect conductance and electroluminescence data using a scanning tunneling microscope (STM) equipped with a custom spectrometer. Through experimental analysis and electronic structure calculations, we provide evidence for a molecule-electrode interfacial exciton coupled to a junction cavity plasmon. Importantly, we find that close to resonant transport conditions, the molecular junction functions as a single emitter that is strongly coupled to the junction cavity mode, leading to characteristic Rabi splitting of the emission spectrum and providing the first example of an electroluminescence-driven single-molecule system in the regime of strong light-matter coupling.

TeNPy (short for ‘Tensor Network Python’) is a python library for the simulation of strongly correlated quantum systems with tensor networks. The philosophy of this library is to achieve a balance of readability and usability for new-comers, while at the same time providing powerful algorithms for experts. The focus is on MPS algorithms for 1D and 2D lattices, such as DMRG ground state search, as well as dynamics using TEBD, TDVP, or MPO evolution. This article is a companion to the recent version 1.0 release of TeNPy and gives a brief overview of the package.

TeNPy (short for ‘Tensor Network Python’) is a python library for the simulation of strongly correlated quantum systems with tensor networks. The philosophy of this library is to achieve a balance of readability and usability for new-comers, while at the same time providing powerful algorithms for experts. The focus is on MPS algorithms for 1D and 2D lattices, such as DMRG ground state search, as well as dynamics using TEBD, TDVP, or MPO evolution. This article is a companion to the recent version 1.0 release of TeNPy and gives a brief overview of the package.

Recent case-by-case studies revealed that the dispersion of low-energy excitations in gapless frustration-free Hamiltonians is often quadratic or softer. In this paper, we argue that this is actually a general property of such systems. By combining the previous study by Bravyi and Gosset and the min-max principle, we prove this hypothesis for models with local Hilbert spaces of dimension two that contains only nearest-neighbor interactions on cubic lattice. This may be understood as a no-go theorem realizing gapless phases with linearly dispersive excitations in frustration-free Hamiltonians. We also provide examples of frustration-free Hamiltonians in which the plane-wave state of a single spin flip does not constitute low-energy excitations.

Anomalous Hall crystals (AHCs) form a new phase of matter with spontaneous crystallization and quantized Hall response. It has been invoked to explain a recent experiment on rhombohedral pentalayer graphene, but a simple conceptual understanding of its existence has been lacking. Here, the authors propose a simple three-patch model that captures how quantum mechanical exchange interactions can stabilize the AHC phase, and apply it to analyze the phenomenology of rhombohedral pentalayer graphene.

Recent experiments on rhombohedral pentalayer graphene with a substrate-induced moiré potential have identified both Chern insulators and fractional quantum Hall states at zero magnetic field. Surprisingly, these states are observed in strong displacement fields where the effects of the moiré lattice are weak, and seem to be readily accessed without fine-tuning. To address these experimental puzzles, we study a model of interacting electrons in this geometry. Within self-consistent Hartree-Fock (SCHF) calculations, we find an isolated Chern band with small bandwidth and good quantum geometry. Exact diagonalization and density-matrix renormalization group calculations both confirm the band hosts fractional quantum Hall states without a magnetic field. Remarkably, the Chern band is stable at a wide range of angles, at four through six rhombohedral layers, at varying rhombohedral hopping parameters, and-most strikingly-survives in SCHF calculations when the moiré potential vanishes. In this limit, the state spontaneously breaks time-reversal and translation symmetry simultaneously, giving a topological crystalline state that we term the "anomalous Hall crystal." We argue this is a general mechanism to create stable Chern bands in rhombohedral multilayer graphene, opening the door to studying the interplay between electronic topology, fractionalization, and spontaneous translation symmetry breaking.

We investigate the Berezinskii-Kosterlitz-Thouless (BKT) transition in a semiconductor-superconductor two-dimensional Josephson junction array. Tuned by an electrostatic top gate, the system exhibits separate superconducting (S), anomalous metal (M*), and insulating (I) phases, bordered by separatrices of the temperature-dependent sheet resistance Rs. We find that the gate-dependent BKT transition temperature falls to zero at the S-M* boundary, suggesting incomplete vortex-antivortex pairing in the M* phase. In the S phase, Rs is roughly proportional to the perpendicular magnetic field at the BKT transition, as expected, while in the M* phase, Rs deviates from its zero-field value as a power law in the field with exponent close to 1/2 at low temperature. An in-plane magnetic field eliminates the M* phase, leaving a small scaling exponent at the S-I boundary, which we interpret as a remnant of the incipient M* phase.

It is shown that the stroboscopic time evolution under a Floquet unitary, in any spatial dimension, and of any Hermitian operator, can be mapped to an operator Krylov space, which is identical to that generated by the edge operator of the noninteracting Floquet transverse-field Ising model (TFIM) in one-spatial dimension, and with inhomogeneous Ising and transverse field couplings. The latter has four topological phases reflected by the absence (topologically trivial) or presence (topologically nontrivial) of edge modes at 0 and/or π quasienergies. It is shown that the Floquet dynamics share certain universal features characterized by how the Krylov parameters vary in the topological phase diagram of the Floquet TFIM with homogeneous couplings. These results are highlighted through examples, all chosen for numerical convenience to be in one spatial dimension: nonintegrable Floquet spin $1/2$ chains and Floquet Z3 clock model where the latter hosts period-tripled edge modes.

Majorana bound states (MBSs) are quasiparticles that are their own antiparticles. They are predicted to emerge as zero-energy modes localized at the boundary of a topological superconductor. No intrinsic topological superconductor is known to date. However, by interfacing conventional superconductors and semiconductors with strong spin-orbit coupling, it is possible to create a system hosting topological states. Hence, epitaxial superconductors and semiconductors have emerged as an attractive material system with atomically sharp interfaces and broad flexibility in device fabrications incorporating Josephson junctions. We discuss the basics of topological superconductivity and provide insight into how to go beyond current state-of-the-art experiments. We argue that the ultimate success in realizing MBS physics requires the observation of non-Abelian braiding and fusion experiments. Published by the American Physical Society 2024

Results are presented for the dynamics of edge modes in interacting Floquet Ising chains. It is shown that in addition to the quasistable 0 and π edge modes, a third long lived edge mode arising from the operator product of the 0 and π edge modes exists. Depending on the microscopic parameters, this Floquet product mode is shown to have a substantially longer lifetime than the individual 0 and π modes. This is triggered by a scattering process which converts a 0 mode into a π mode while scattering two bulk excitations. This process can lead to a rapid decay of both 0 and π mode without affecting the product mode.

Dynamic critical fluctuations in magnetic materials encode important information about magnetic ordering in the associated critical exponents. Using nitrogen-vacancy centers in diamond, we implement T2 (spin-decoherence) noise magnetometry to study critical dynamics in a 2D Van der Waals magnet CrSBr. By analyzing NV decoherence on time scales approaching the characteristic correlation time τc of critical fluctuations, we extract the critical exponent $ν$ for the correlation length. Our result deviates from the Ising prediction and highlights the role of long-range dipolar interactions in 2D CrSBr. Furthermore, analyzing the divergence of the correlation length suggests the possibility of 2D-XY criticality in CrSBr in a temperature window near TC where static magnetic domains are absent. Our work provides a first demonstration of T2 noise magnetometry to quantitatively analyze critical scaling behavior in 2D materials.

The physics of superconductivity in magic-angle twisted bilayer graphene (MATBG) is a topic of keen interest in moiré systems research, and it may provide insight into the pairing mechanism of other strongly correlated materials such as high-Tc superconductors. Here, we use DC-transport and microwave circuit quantum electrodynamics (cQED) to measure directly the superfluid stiffness of superconducting MATBG via its kinetic inductance. We find the superfluid stiffness to be much larger than expected from conventional Fermi liquid theory; rather, it is comparable to theoretical predictions involving quantum geometric effects that are dominant at the magic angle. The temperature dependence of the superfluid stiffness follows a power-law, which contraindicates an isotropic BCS model; instead, the extracted power-law exponents indicate an anisotropic superconducting gap, whether interpreted within the Fermi liquid framework or by considering quantum geometry of flat-band superconductivity. Moreover, a quadratic dependence of the superfluid stiffness on both DC and microwave current is observed, which is consistent with Ginzburg-Landau theory. Taken together, our findings indicate that MATBG is an unconventional superconductor with an anisotropic gap and strongly suggest a connection between quantum geometry, superfluid stiffness, and unconventional superconductivity in MATBG. The combined DC-microwave measurement platform used here is applicable to the investigation of other atomically thin superconductors.

Abstract The exploration of emerging quantum phenomena by stacking dissimilar atomic layered materials into van der Waals (vdW) heterostructures has driven the development of layer assembly techniques. Achieving ultralow disorder within these heterostructures is crucial for unlocking their novel physical properties. However, current fabrication methods for designer heterostructures have limitations in throughput, yield, and scalability. Over the past decade, engineering toolkits have evolved to address some of these challenges, but their adoption for fabricating designer heterostructures remains limited. In this review, an overview of these emerging engineering toolkits is provided, and examine their utility and limitations in achieving ultralow disordered heterostructures. It is hoped that the insights from this review article can help guide future research directions on advancing the fabrication process of designer heterostructures.

The tunneling of Cooper pairs across a Josephson junction (JJ) allows for the nonlinear inductance necessary to construct superconducting qubits, amplifiers, and various other quantum circuits. An alternative approach using hybrid superconductor-semiconductor JJs can enable superconducting qubit architectures with all electric control. Here we present continuous-wave and time-domain characterization of gatemon qubits and coplanar waveguide resonators based on an InAs two-dimensional electron gas. We show that the qubit undergoes a vacuum Rabi splitting with a readout cavity, and we drive coherent Rabi oscillations between the qubit ground and first excited states. We measure qubit relaxation times to be T 1 = 100 ns over a 1.5 GHz tunable band. We detail the loss mechanisms present in these materials through a systematic study of the quality factors of coplanar waveguide resonators. While various loss mechanisms are present in III-V gatemon circuits, we detail future directions in enhancing the relaxation times of qubit devices on this platform. Published by the American Physical Society 2024

We study a periodically driven one-dimensional Kitaev model in the presence of disorder. In the clean limit our model exhibits four topological phases corresponding to the existence or nonexistence of edge modes at zero and π quasienergy. When potential disorder is added, the system parameters get renormalized and the system may exhibit a topological phase transition. When starting from the Majorana π mode (MPM) phase, which hosts only edge Majoranas with quasienergy π, disorder induces a transition into a neighboring phase with both π and zero modes on the edges. We characterize the disordered system using (i) exact diagonalization, (ii) Arnoldi mapping onto an effective tight-binding chain, and (iii) topological entanglement entropy.

Recent research has revealed remarkable properties of the two-dimensional (2D) van der Waals layered crystal CrSBr, which is both a semiconductor and an $A$-type antiferromagnet. Here we show the role of strong magnetoelastic coupling in the generation and propagation of coherent magnons in CrSBr. Time- and spatially resolved magneto-optical Kerr effect microscopy reveals two time-varying transient strain fields induced by out-of-plane transverse and in-plane longitudinal lattice displacements. These transient strain fields launch coherent wavepackets of magnons, optical and acoustic, at 24.6±0.8 and 33.4±0.50.16em0exGHz, respectively. These findings suggest mechanisms for controlling and manipulating coherent magnons from distinct magnetoelastic couplings in this 2D van der Waals magnetic semiconductor.

We investigate the interplay between the quantum Hall (QH) effect and superconductivity in InAs surface quantum well (SQW)/NbTiN heterostructures using a quantum point contact (QPC). We use QPC to control the proximity of the edge states to the superconductor. By measuring the upstream and downstream resistances of the device, we investigate the efficiency of Andreev conversion at the InAs/NbTiN interface. Our experimental data is analyzed using the Landauer-B\"uttiker formalism, generalized to allow for Andreev reflection processes. We show that by varying the voltage of the QPC, VQPC, the average Andreev reflection, $A$, at the QH-SC interface can be tuned from 50% to ∼10%. The evolution of $A$ with VQPC extracted from the measurements exhibits plateaus separated by regions for which $A$ varies continuously with VQPC. The presence of plateaus suggests that for some ranges of VQPC the QPC might be pinching off almost completely from the QH-SC interface some of the edge modes. Our work shows an experimental setup to control and advance the understanding of the complex interplay between superconductivity and QH effect in two-dimensional gas systems.

We investigate the effects of an in-plane magnetic field on the weak antilocalization signature of near-surface quantum wells lacking bulk and inversion symmetry. The measured magnetoconductivity, which is conductivity as a function of the out-of-plane magnetic field, exhibits a strong anisotropy with respect to the direction of the in-plane magnetic field. The twofold symmetry of the observed magnetoanisotropy originates from the competition between Rashba and Dresselhaus spin-orbit couplings. The high sensitivity of the weak antilocalization to the spin texture produced by the combined Zeeman and spin-orbit fields results in very large anisotropy ratios, reaching 100%. Using a semiclassical universal model in quantitative agreement with the experimental data, we uniquely determine the values of the Dresselhaus and Rashba parameters as well as the effective in-plane g-factor of the electrons. Understanding these parameters provides prospects for different applications ranging from spintronics to topological quantum computing. Published by the American Physical Society 2024

Quenched disorder slows down the scrambling of quantum information. Using a bottom-up approach, we formulate a kinetic theory of scrambling in a correlated metal near a superconducting transition, following the scrambling dynamics as the impurity scattering rate is increased. Within this framework, we rigorously show that the butterfly velocity $v$ is bounded by the light-cone velocity vlc set by the Fermi velocity. We analytically identify a disorder-driven dynamical transition occurring at small but finite disorder strength between a spreading of information characterized at late times by a discontinuous shock wave propagating at the maximum velocity vlc, and a smooth traveling wave belonging to the Fisher or Kolmogorov-Petrovsky-Piskunov (FKPP) class and propagating at a slower, if not considerably slower, velocity $v$. In the diffusive regime, we establish the relation v²/λFKPP∼Del, where λFKPP is the Lyapunov exponent set by the inelastic scattering rate and Del is the elastic diffusion constant.

We investigate twisted bilayer graphene (TBG) at filling ν=-3 in the presence of realistic heterostrain. Strain amplifies the band dispersion and drives the system beyond the strong-coupling regime of previous theoretical studies. We use DMRG to conduct an unbiased, large-scale numerical calculations that include all spin and valley degrees of freedom, up to bond dimension χ=240.16em0ex576. We establish a global phase diagram that unifies a number of theoretical and experimental results. Near zero strain we find an intervalley-coherent quantized anomalous Hall (QAH-IVC) state, a competitive strong-coupling order that evaded past numerical studies. A tiny strain around $0.05%$ drives a transition into an incommensurate Kekul\'e spiral (IKS) phase, supporting the mean-field prediction in [Kwan et al., Phys. Rev. X 11, 041063 (2021)]. Even higher strains above $0.2%$ favor a flavor-symmetric metallic order, which may explain metals found at ν=-3 in many experiments.

It is shown that the stroboscopic time-evolution under a Floquet unitary, in any spatial dimension, and of any Hermitian operator, can be mapped to an operator Krylov space which is identical to that generated by the edge operator of the non-interacting Floquet transverse-field Ising model (TFIM) in one-spatial dimension, and with inhomogeneous Ising and transverse field couplings. The latter has four topological phases reflected by the absence (topologically trivial) or presence (topologically non-trivial) of edge modes at $0$ and/or $π$ quasi-energies. It is shown that the Floquet dynamics share certain universal features characterized by how the Krylov parameters vary in the topological phase diagram of the Floquet TFIM with homogeneous couplings. These results are highlighted through examples, all chosen for numerical convenience to be in one spatial dimension: non-integrable Floquet spin $1/2$ chains and Floquet Z3 clock model where the latter hosts period-tripled edge modes.

The performance of crystalline organic semiconductors depends on the solid-state structure, especially the orientation of the conjugated components with respect to device platforms. Often, crystals can be engineered by modifying chromophore substituents through synthesis. Meanwhile, dissymetry is necessary for high-tech applications like chiral sensing, optical telecommunications, and data storage. The synthesis of dissymmetric molecules is a labor-intensive exercise that might be undermined because common processing methods offer little control over orientation. Crystal twisting has emerged as a generalizable method for processing organic semiconductors and offers unique advantages, such as patterning of physical and chemical properties and chirality that arises from mesoscale twisting. The precession of crystal orientations can enrich performance because achiral molecules in achiral space groups suddenly become candidates for the aforementioned technologies that require dissymetry.

The sudden depinning of vortices with increasing current through a super-semihybrid Josephson junction array results in a burst of differential resistance at integer and half-integer peaks of critical current. A striking feature is the split feature at $f=0$, indicating the absence of vortices at precisely zero field. The flat-topped portion at $f=1/2$ and the slanted top part at $f=1$ also reveal features of how the dynamical transition occurs.

The transverse field Ising model (TFIM) on the half-infinite chain possesses an edge zero mode. This work considers an impurity model: TFIM perturbed by a boundary integrability-breaking interaction. For sufficiently large transverse field, but in the ordered phase of the TFIM, the zero mode is observed to decay. The decay is qualitatively different from zero modes where the integrability-breaking interactions are nonzero all along the chain. It is shown that for the impurity model, the zero mode decays by relaxing to a nonlocal quasiconserved operator, the latter being exactly conserved when the opposite edge of the chain has no noncommuting perturbations so as to ensure perfect degeneracy of the spectrum. In the thermodynamic limit, the quasiconserved operator vanishes, and a regime is identified where the decay of the zero mode obeys Fermi's golden rule. A toy model for the decay is constructed in Krylov space and it is highlighted how Fermi's golden rule may be recovered from this toy model.

Abstract Ultra-thin films of low damping ferromagnetic insulators with perpendicular magnetic anisotropy have been identified as critical to advancing spin-based electronics by significantly reducing the threshold for current-induced magnetization switching while enabling new types of hybrid structures or devices. Here, we have developed a new class of ultra-thin spinel structure Li0.5Al1.0Fe1.5O4 (LAFO) films on MgGa2O4 (MGO) substrates with: 1) perpendicular magnetic anisotropy; 2) low magnetic damping and 3) the absence of degraded or magnetic dead layers. These films have been integrated with epitaxial Pt spin source layers to demonstrate record low magnetization switching currents and high spin-orbit torque efficiencies. These LAFO films on MGO thus combine all of the desirable properties of ferromagnetic insulators with perpendicular magnetic anisotropy, opening new possibilities for spin based electronics.

We formulate a kinetic theory of quantum information scrambling in the context of a paradigmatic model of interacting electrons in the vicinity of a superconducting phase transition. We carefully derive a set of coupled partial differential equations that effectively govern the dynamics of information spreading in generic dimensions. Their solutions show that scrambling propagates at the maximal speed set by the Fermi velocity. At early times, we find exponential growth at a rate set by the inelastic scattering. At late times, we find that scrambling is governed by shock-wave dynamics with traveling waves exhibiting a discontinuity at the boundary of the light cone. Notably, we find perfectly causal dynamics where the solutions do not spill outside of the light cone.

Abstract Adoption of fast, parametric coupling elements has improved the performance of superconducting qubits, enabling recent demonstrations of quantum advantage in randomized sampling problems. The development of low loss, high contrast couplers is critical for scaling up these systems. We present a blueprint for a gate-tunable coupler realized with a two-dimensional electron gas in an InAs/InGaAs heterostructure. Rigorous numerical simulations of the semiconductor and high frequency electromagnetic behavior of the coupler and microwave circuitry yield an on/off ratio of more than one order of magnitude. We give an estimate of the dielectric-limited loss from the inclusion of the coupler in a two qubit system, with coupler coherences ranging from a few to tens of microseconds.

We study quantum transport and AC Josephson effect of hexagonal boron nitride encapsulated graphene (BGB) Josephson junctions (JJs). Our experiments reveal the emergence of the half-integer Shapiro steps in the n-type regime with high electron carrier densities. We attribute this observation to the gate-tunable transmission probability of the graphene junction. Our numerical simulations are consistent with the appearance of half-integer Shapiro steps at high transparency, which suggests a skewed current phase relationship in the graphene JJ.

In recent years, correlated insulating states, unconventional superconductivity, and topologically non-trivial phases have all been observed in several moiré heterostructures. However, understanding of the physical mechanisms behind these phenomena is hampered by the lack of local electronic structure data. Here, we use scanning tunnelling microscopy and spectroscopy to demonstrate how the interplay between correlation, topology, and local atomic structure determines the behaviour of electron-doped twisted monolayer-bilayer graphene. Through gate- and magnetic field-dependent measurements, we observe local spectroscopic signatures indicating a quantum anomalous Hall insulating state with a total Chern number of ±2 at a doping level of three electrons per moiré unit cell. We show that the sign of the Chern number and associated magnetism can be electrostatically switched only over a limited range of twist angle and sample hetero-strain values. This results from a competition between the orbital magnetization of filled bulk bands and chiral edge states, which is sensitive to strain-induced distortions in the moiré superlattice.

Twisted bilayer graphene (TBG) has garnered significant interest in condensed matter physics over the past few years. Here, the authors present numerical investigations of TBG implementing state-of-the-art quantum chemistry methods. Using a gauge-invariant order parameter, they show a C2z\ensuremath{\mathcal{T}} phase transition at charge neutrality which persists at noninteger fillings near charge neutrality. The work is the first systematic study of TBG for noninteger fillings near charge neutrality.

The transverse field Ising model (TFIM) on the half-infinite chain possesses an edge zero mode. This work considers an impurity model -- TFIM perturbed by a boundary integrability breaking interaction. For sufficiently large transverse field, but in the ordered phase of the TFIM, the zero mode is observed to decay. The decay is qualitatively different from zero modes where the integrability breaking interactions are non-zero all along the chain. It is shown that for the impurity model, the zero mode decays by relaxing to a non-local quasi-conserved operator, the latter being exactly conserved when the opposite edge of the chain has no non-commuting perturbations so as to ensure perfect degeneracy of the spectrum. In the thermodynamic limit, the quasi-conserved operator vanishes, and a regime is identified where the decay of the zero mode obeys Fermi's Golden Rule. A toy model for the decay is constructed in Krylov space and it is highlighted how Fermi's Golden Rule may be recovered from this toy model.

Quenched disorder slows down the scrambling of quantum information. Using a bottom-up approach, we formulate a kinetic theory of scrambling in a correlated metal near a superconducting transition, following the scrambling dynamics as the impurity scattering rate is increased. Within this framework, we rigorously show that the butterfly velocity $v$ is bounded by the light cone velocity v lc set by the Fermi velocity. We analytically identify a disorder-driven dynamical transition occurring at small but finite disorder strength between a spreading of information characterized at late times by a discontinuous shock wave propagating at the maximum velocity v lc, and a smooth traveling wave belonging to the Fisher or Kolmogorov-Petrovsky-Piskunov (FKPP) class and propagating at a slower, if not considerably slower, velocity $v$. In the diffusive regime, we establish the relation v²/λ FKPP ∼ D el where λ FKPP is the Lyapunov exponent set by the inelastic scattering rate and D el is the elastic diffusion constant.

Spin-Hall nano-oscillators (SHNOs) are promising spintronic devices to realize current controlled GHz frequency signals in nanoscale devices for neuromorphic computing and creating Ising systems. However, traditional SHNOs devices based on transition metals have high auto-oscillation threshold currents as well as low quality factors and output powers. Here we demonstrate a new type of hybrid SHNO based on a permalloy (Py) ferromagnetic-metal nanowire and low-damping ferrimagnetic insulator, in the form of epitaxial lithium aluminum ferrite (LAFO) thin films. The superior characteristics of such SHNOs are associated with the excitation of larger spin-precession angles and volumes. We further find that the presence of the ferrimagnetic insulator enhances the auto-oscillation amplitude of spin-wave edge modes, consistent with our micromagnetic modeling. This hybrid SHNO expands spintronic applications, including providing new means of coupling multiple SHNOs for neuromorphic computing and advancing magnonics.

Abstract Optoelectronic properties of anisotropic crystals vary with direction requiring that the orientation of molecular organic semiconductor crystals is controlled in optoelectronic device active layers to achieve optimal performance. Here, a generalizable strategy to introduce periodic variations in the out‐of‐plane orientations of 5,11‐bis(triisopropylsilylethynyl)anthradithiophene (TIPS ADT) crystals is presented. TIPS ADT crystallized from the melt in the presence of 16 wt.% polyethylene (PE) forms banded spherulites of crystalline fibrils that twist in concert about the radial growth direction. These spherulites exhibit band‐dependent light absorption, photoluminescence, and Raman scattering depending on the local orientation of crystals. Mueller matrix imaging reveals strong circular extinction (CE), with TIPS ADT banded spherulites exhibiting domains of positive or negative CE signal depending on the crystal twisting sense. Furthermore, orientation‐dependent enhancement in charge injection and extraction in films of twisted TIPS ADT crystals compared to films of straight crystals is visualized in local conductive atomic force microscopy maps. This enhancement leads to 3.3‐ and 6.2‐times larger photocurrents and external quantum efficiencies, respectively, in photodetectors comprising twisted crystals than those comprising straight crystals.

Antisymmetric exchange interactions lead to nonreciprocal spin-wave propagation. As a result, spin waves confined in a nanostructure are not standing waves; they have a time-dependent phase, because counterpropagating waves of the same frequency have different wavelengths. We report on a Brillouin light scattering (BLS) study of confined spin waves in Co/Pt nanowires with strong Dzyaloshinskii-Moriya interactions. Spin-wave quantization in narrow (200-nm-wide) wires dramatically reduces the frequency shift between BLS Stokes and anti-Stokes lines associated with the scattering of light incident transverse to the nanowires. In contrast, the BLS frequency shift associated with the scattering of spin waves propagating along the nanowire length is independent of nanowire width. A model that considers the chiral nature of modes captures this physics and predicts a dramatic reduction in frequency shift of light scattered from higher-energy spin waves in narrow wires, which is confirmed by our experiments.

Guiding many-body systems to desired states is a central challenge of modern quantum science, with applications from quantum computation1,2 to many-body physics3 and quantum-enhanced metrology4. Approaches to solving this problem include step-by-step assembly5,6, reservoir engineering to irreversibly pump towards a target state7,8 and adiabatic evolution from a known initial state9,10. Here we construct low-entropy quantum fluids of light in a Bose-Hubbard circuit by combining particle-by-particle assembly and adiabatic preparation. We inject individual photons into a disordered lattice for which the eigenstates are known and localized, then adiabatically remove this disorder, enabling quantum fluctuations to melt the photons into a fluid. Using our platform11, we first benchmark this lattice melting technique by building and characterizing arbitrary single-particle-in-a-box states, then assemble multiparticle strongly correlated fluids. Intersite entanglement measurements performed through single-site tomography indicate that the particles in the fluid delocalize, whereas two-body density correlation measurements demonstrate that they also avoid one another, revealing Friedel oscillations characteristic of a Tonks-Girardeau gas12,13. This work opens new possibilities for the preparation of topological and otherwise exotic phases of synthetic matter3,14,15.

Transparent contact interfaces in superconductor–graphene hybrid systems are critical for realizing superconducting quantum applications. Here, we examine the effect of the edge contact fabrication process on the transparency of the superconducting aluminum–graphene junction. We show significant improvement in the transparency of our superconductor–graphene junctions by promoting the chemical component of the edge contact etch process. Our results compare favorably with state-of-the-art graphene Josephson junctions. The findings of our study contribute to advancing the fabrication knowledge of edge-contacted superconductor–graphene junctions.

Moiré systems made from stacked two-dimensional materials host novel correlated and topological states that can be electrically controlled via applied gate voltages. We have used this technique to manipulate Chern domains in an interaction-driven quantum anomalous Hall insulator made from twisted monolayer-bilayer graphene (tMBLG). This has allowed the wavefunction of chiral interface states to be directly imaged using a scanning tunneling microscope (STM). To accomplish this tMBLG carrier concentration was tuned to stabilize neighboring domains of opposite Chern number, thus providing topological interfaces completely devoid of any structural boundaries. STM tip pulse-induced quantum dots were utilized to induce new Chern domains and thereby create new chiral interface states with tunable chirality at predetermined locations. Theoretical analysis confirms the chiral nature of observed interface states and enables the determination of the characteristic length scale of valley polarization reversal across neighboring tMBLG Chern domains. tMBLG is shown to be a useful platform for imaging the exotic topological properties of correlated moiré systems.

When the two layers of a twisted moiré system are subject to different degrees of strain, the effect is amplified by the inverse twist angle, e.g., by a factor of 50 in magic angle twisted bilayer graphene (TBG). Samples of TBG typically have heterostrains of 0.1-0.7%, increasing the bandwidth of the "flat'' bands by as much as tenfold, placing TBG in an intermediate coupling regime. Here we study the phase diagram of TBG in the presence of heterostrain with unbiased, large-scale density matrix renormalization group calculations (bond dimension $χ=24576$), including all spin and valley degrees of freedom. Working at filling $ν= -3$, we find a strain of 0.05% drives a transition from a quantized anomalous Hall insulator into an incommensurate-Kekulé spiral (IKS) phase. This peculiar order, proposed and studied at mean-field level by Kwan et al (PRX 11, 041063), breaks both valley conservation and translation symmetry T, but preserves a modified translation symmetry T' with moiré-incommensurate phase modulation. Even higher strains drive the system to a fully symmetric metal.

A growing body of experimental work suggests that magic angle twisted bilayer graphene exhibits a "cascade" of spontaneous symmetry-breaking transitions, sparking interest in the potential relationship between symmetry breaking and superconductivity. However, it has proven difficult to find experimental probes which can unambiguously identify the nature of the symmetry breaking. Here, we show how atomically resolved scanning tunneling microscopy can be used as a fingerprint of symmetry-breaking order. By analyzing the pattern of sublattice polarization and "Kekulé" distortions in small magnetic fields, order parameters for each of the most competitive symmetry-breaking states can be identified. In particular, we show that the "Kramers intervalley coherent state," which theoretical work predicts to be the ground state at even integer fillings, shows a Kekulé distortion which emerges only in a magnetic field.

Weyl semimetals can emerge from Dirac semimetals when the time-reversal or spatial-inversion symmetries are broken. Recently, it has been proposed based on the Floquet theory that Dirac semimetals can be converted into Weyl semimetals even by shining circularly polarized light (CPL). Here we have investigated the possibility of such a Dirac-Weyl conversion by measuring the CPL-induced anomalous Hall conductivity (AHC) in a massive 3D Dirac semimetal Co3Sn2S2 in the paramagnetic phase using ultrafast mid-infrared pump-terahertz Faraday rotation probe spectroscopy. We find that the field-strength and driving frequency dependence of the observed AHC is well accounted for by CPL-induced nonzero Berry curvature associated with the splitting of the Dirac bands as predicted by the Floquet theory. The estimated splitting of the Dirac bands reaches about 60 % of the mass gap and the calculated CPL-induced AHC quantitatively reproduces the experimental observation, demonstrating a promising route toward the realization of Floquet-Weyl states from massive Dirac semimetals.

The anomalous Hall effect, a hallmark of broken time-reversal symmetry and spin–orbit coupling, is frequently observed in magnetically polarized systems. However, its realization in nominally non-magnetic systems remains elusive. Here, we report on the observation of the anomalous Hall effect in nominally non-magnetic KTaO3. Anomalous Hall effect emerges in reduced KTaO3 and shows an extrinsic to intrinsic crossover. A paramagnetic behavior is observed in reduced samples and confirmed using first principles calculations. The observed anomalous Hall effect follows the oxygen vacancy-induced magnetization response, suggesting that the localized magnetic moments of the oxygen vacancies scatter conduction electrons asymmetrically and give rise to the anomalous Hall effect. The anomalous Hall conductivity is found to be insensitive to the scattering rate in the low temperature limit (T < 5 K), implying that the Berry curvature of the electrons on the Fermi surface controls the anomalous Hall effect. Our observations provide a detailed picture of many-body interactions, which trigger the anomalous Hall effect in a non-magnetic system.

Hybrid superconductor–semiconductor heterostructures are a promising platform for quantum devices based on mesoscopic and topological superconductivity. In these structures, a semiconductor must be in close proximity to a superconductor and form an Ohmic contact. This can be accommodated in narrow bandgap semiconductors, such as InAs, where the surface Fermi level is positioned close to the conduction band. In this work, we study the structural properties of near-surface InAs quantum wells and find that surface morphology is closely connected to low-temperature transport, where electron mobility is highly sensitive to the growth temperature of the underlying graded buffer layer. By introducing an In0.81Al0.19As capping layer, we show that we change the surface Fermi level pinning of the In0.81Al0.19As thin film as compared to the In0.81Ga0.19As, giving rise to a tuning of the Fermi level in the InAs layer. Experimental measurements show a strong agreement with Schrödinger–Poisson calculations of the electron density, suggesting the conduction band energy of the In0.81Ga0.19As and In0.81Al0.19As surface is pinned to 40 and 309 meV above the Fermi level, respectively.

Switching of perpendicular magnetization via spin–orbit torque (SOT) is of particular interest in the development of non-volatile magnetic random access memory (MRAM) devices. We studied current-induced magnetization switching of Ir/GdFeCo/Cu/Pt heterostructures in a Hall cross geometry as a function of the in-plane applied magnetic field. Remarkably, magnetization switching is observed at zero applied field. This is shown to result from the competition between SOT, the Oersted field generated by the charge current, and the material's coercivity. Our results show a means of achieving zero-field switching that can impact the design of future spintronics devices, such as SOT-MRAM.

Many molecular crystals (approximately one third) grow as twisted, helicoidal ribbons from the melt, and this preponderance is even higher in restricted classes of materials, for instance, charge-transfer complexes. Previously, twisted crystallites of such complexes present an increase in carrier mobilities. Here, the effect of twisting on charge mobility is better analyzed for a monocomponent organic semiconductor, 2,5-bis(3-dodecyl-2-thienyl)-thiazolo[5,4-d]thiazole (BDT), that forms twisted crystals with varied helicoidal pitches and makes possible a correlation of twist strength with carrier mobility. Films are analyzed by X-ray scattering and Mueller matrix polarimetry to characterize the microscale organization of the polycrystalline ensembles. Carrier mobilities of organic field-effect transistors are five times higher when the crystals are grown with the smallest pitches (most twisted), compared to those with the largest pitches, along the fiber elongation direction. A tenfold increase is observed along the perpendicular direction. Simulation of electrical potential based on scanning electron microscopy images and density functional theory suggests that the twisting-enhanced mobility is mainly controlled by the fiber organization in the film. A greater number of tightly packed twisted fibers separated by numerous smaller gaps permit better charge transport over the film surface compared to fewer big crystallites separated by larger gaps.

We investigate the effects of an in-plane magnetic field on the weak antilocalization signature of near-surface quantum wells lacking bulk and inversion symmetry. The measured magnetoconductivity exhibits a strong anisotropy with respect to the direction of the in-plane magnetic field. The two-fold symmetry of the observed magneto-anisotropy originates from the competition between Rashba and Dresselhaus spin-orbit couplings. The high sensitivity of the weak antilocalization to the spin texture produced by the combined Zeeman and spin-orbit fields results in very large anisotropy ratios, reaching 100%. Using a semiclassical universal model in quantitative agreement with the experimental data, we uniquely determine the values of the Dresselhaus and Rashba parameters as well as the effective in-plane g-factor of the electrons. Understanding these parameters provides new prospects for novel applications ranging from spintronics to topological quantum computing.

Cavity quantum electrodynamics, which explores the granularity of light by coupling a resonator to a nonlinear emitter1, has played a foundational role in the development of modern quantum information science and technology. In parallel, the field of condensed matter physics has been revolutionized by the discovery of underlying topological2–4, often arising from the breaking of time-reversal symmetry, as in the case of the quantum Hall effect. In this work, we explore the cavity quantum electrodynamics of a transmon qubit in a topologically nontrivial Harper–Hofstadter lattice5. We assemble the lattice of niobium superconducting resonators6 and break time-reversal symmetry by introducing ferrimagnets7 before coupling the system to a transmon qubit. We spectroscopically resolve the individual bulk and edge modes of the lattice, detect Rabi oscillations between the excited transmon and each mode and measure the synthetic-vacuum-induced Lamb shift of the transmon. Finally, we demonstrate the ability to employ the transmon to count individual photons8 within each mode of the topological band structure. This work opens the field of experimental chiral quantum optics9, enabling topological many-body physics with microwave photons 10,11 and providing a route to backscatter-resilient quantum communication. Edge modes in chiral topological systems can carry quantum information without backscattering. A topological lattice of superconducting resonators has been coupled to a qubit, providing a platform for chiral quantum electrodynamics and communication.

Skyrmion racetrack memories are highly attractive for next-generation data storage technologies. Skyrmions are noncollinear spin textures stabilized by chiral interactions. To achieve a fast-operating memory device, it is critical to move skyrmions at high speeds. The skyrmion dynamics induced by spin–orbit torques (SOTs) in the commonly studied ferromagnetic films is hindered by strong pinning effects and a large skyrmion Hall effect causing deflection of the skyrmion toward the racetrack edge, which can lead to information loss. Here, we investigate the current-induced nucleation and motion of skyrmions in ferrimagnetic Pt/CoGd/(W or Ta) thin films. We first reveal field-free skyrmion nucleation mediated by Joule heating. We then achieve fast skyrmion motion driven by SOTs with velocities as high as 610 m s –1 and a small skyrmion Hall angle |θ SkHE | ≲ 3°. Our results show that ferrimagnets are better candidates for fast skyrmion-based memory devices with low risk of information loss.

Indium arsenide (InAs) near surface quantum wells (QWs) are promising for the fabrication of semiconductor-superconductor heterostructures given that they allow for a strong hybridization between the two-dimensional states in the quantum well and the ones in the superconductor. In this work, we present results for InAs QWs in the quantum Hall regime placed in proximity of superconducting NbTiN. We observe a negative downstream resistance with a corresponding reduction of Hall (upstream) resistance, consistent with a very high Andreev conversion. We analyze the experimental data using the Landauer-Büttiker formalism, generalized to allow for Andreev reflection processes. We attribute the high efficiency of Andreev conversion in our devices to the large transparency of the InAs/NbTiN interface and the consequent strong hybridization of the QH edge modes with the states in the superconductor.

Gapped two-dimensional topological phases can feature ungappable edge states which are robust even in the absence of protecting symmetries. In this Letter we argue that a multipartite entanglement measure recently proposed in the context of holography, the Markov gap, provides a universal diagnostic of ungappable edge states. Defined as a difference of the reflected entropy and mutual information h(A:B)=SR(A:B)-I(A:B) between two parties, we argue that for $A,B$ being adjacent subregions in the bulk h=c+3ln0.16em0ex2, where c+ is the minimal total central charge of the boundary theory. As evidence, we prove that $h=0$ for string-net models and numerically verify that h=|C|3ln0.16em0ex2 for a Chern-$C$ insulator. Our Letter establishes a unique bulk entanglement criteria for the presence of a conformal field theory on the boundary.

Neuromorphic computing approaches become increasingly important as we address future needs for efficiently processing massive amounts of data. The unique attributes of quantum materials can help address these needs by enabling new energy-efficient device concepts that implement neuromorphic ideas at the hardware level. In particular, strong correlations give rise to highly non-linear responses, such as conductive phase transitions that can be harnessed for short- and long-term plasticity. Similarly, magnetization dynamics are strongly non-linear and can be utilized for data classification. This Perspective discusses select examples of these approaches and provides an outlook on the current opportunities and challenges for assembling quantum-material-based devices for neuromorphic functionalities into larger emergent complex network systems.

Abstract Electrical switching of antiferromagnets is an exciting recent development in spintronics, which promises active antiferromagnetic devices with high speed and low energy cost. In this emerging field, there is an active debate about the mechanisms of current-driven switching of antiferromagnets. For heavy-metal/ferromagnet systems, harmonic characterization is a powerful tool to quantify current-induced spin-orbit torques and spin Seebeck effect and elucidate current-induced switching. However, harmonic measurement of spin-orbit torques has never been verified in antiferromagnetic heterostructures. Here, we report harmonic measurements in Pt/α-Fe2O3 bilayers, which are explained by our modeling of higher-order harmonic voltages. As compared with ferromagnetic heterostructures where all current-induced effects appear in the second harmonic signals, the damping-like torque and thermally-induced magnetoelastic effect contributions in Pt/α-Fe2O3 emerge in the third harmonic voltage. Our results provide a new path to probe the current-induced magnetization dynamics in antiferromagnets, promoting the application of antiferromagnetic spintronic devices.

Results are presented for Floquet systems in two spatial dimensions where the Floquet driving breaks an effective time-reversal symmetry. The driving protocol also induces flat bands that correspond to anomalous Floquet phases where the Chern number is zero and yet chiral edge modes exist. Analytic expressions for the edge modes, Berry curvature, and orbital magnetization are derived for the flat bands. Results are also presented for the static Haldane model for parameters when the bands are flat. Floquet driving of the same model is shown to give rise to Chern insulators as well as anomalous Floquet phases. The orbital magnetization for these different topological phases are presented and are found to be enhanced at half filling by the broken particle-hole symmetry of the Haldane model.

The effect of spin currents on the magnetic order of insulating antiferromagnets (AFMs) is of fundamental interest and can enable new applications. Toward this goal, characterizing the spin-orbit torques (SOTs) associated with AFM-heavy-metal (HM) interfaces is important. Here we report the full angular dependence of the harmonic Hall voltages in a predominantly easy-plane AFM, epitaxial c-axis oriented α-Fe_{2}O_{3} films, with an interface to Pt. By modeling the harmonic Hall signals together with the α-Fe_{2}O_{3} magnetic parameters, we determine the amplitudes of fieldlike and dampinglike SOTs. Out-of-plane field scans are shown to be essential to determining the dampinglike component of the torques. In contrast to ferromagnetic-heavy-metal heterostructures, our results demonstrate that the fieldlike torques are significantly larger than the dampinglike torques, which we correlate with the presence of a large imaginary component of the interface spin-mixing conductance. Our work demonstrates a direct way of characterizing SOTs in AFM-HM heterostructures.

Heterostructures obtained from layered assembly of 2D materials such as graphene and hexagonal boron nitride have potential in the development of new electronic devices. Whereas various materials techniques can now produce macroscopic scale graphene, the construction of similar size heterostructures with atomically clean interfaces is still unrealized. A primary barrier has been the inability to remove polymeric residues from the interfaces that arise between layers when fabricating heterostructures. Here, the interface cleaning problem of polymer-contaminated heterostructures is experimentally studied from an energy viewpoint. With this approach, it is established that the interface cleaning mechanism involves a combination of thermally activated polymer residue mobilization and their mechanical actuation. This framework allows a systematic approach for fabricating record large-area clean heterostructures from polymer-contaminated graphene. These heterostructures provide state-of-the-art electronic performance. This study opens new strategies for the scalable production of layered materials heterostructures.